Please use this identifier to cite or link to this item:
https://hdl.handle.net/2440/131416
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Type: | Journal article |
Title: | Constructing nitrided interfaces for stabilizing Li metal electrodes in liquid electrolytes |
Author: | Wang, Z. Wang, Y. Wu, C. Pang, W.K. Mao, J. Guo, Z. |
Citation: | Chemical Science, 2021; 12(26):8945-8966 |
Publisher: | Royal Society of Chemistry |
Issue Date: | 2021 |
ISSN: | 2041-6520 2041-6539 |
Statement of Responsibility: | Zhijie Wang, Yanyan Wang, Chao Wu, Wei Kong Pang, Jianfeng Mao and Zaiping Guo |
Abstract: | Traditional Li ion batteries based on intercalation-type anodes have been approaching their theoretical limitations in energy density. Replacing the traditional anode with metallic Li has been regarded as the ultimate strategy to develop next-generation high-energy-density Li batteries. Unfortunately, the practical application of Li metal batteries has been hindered by Li dendrite growth, unstable Li/electrolyte interfaces, and Li pulverization during battery cycling. Interfacial modification can effectively solve these challenges and nitrided interfaces stand out among other functional layers because of their impressive effects on regulating Li+ flux distribution, facilitating Li+ diffusion through the solid-electrolyte interphase, and passivating the active surface of Li metal electrodes. Although various designs for nitrided interfaces have been put forward in the last few years, there is no paper that specialized in reviewing these advances and discussing prospects. In consideration of this, we make a systematic summary and give our comments based on our understanding. In addition, a comprehensive perspective on the future development of nitrided interfaces and rational Li/electrolyte interface design for Li metal electrodes is included. |
Rights: | Open Access Article. Published on 01 June 2021. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence. |
DOI: | 10.1039/d1sc01806j |
Grant ID: | http://purl.org/au-research/grants/arc/LP160101629 http://purl.org/au-research/grants/arc/LE120100104 http://purl.org/au-research/grants/arc/DP200101862 http://purl.org/au-research/grants/arc/DP210101486 http://purl.org/au-research/grants/arc/LE180100141 |
Published version: | http://dx.doi.org/10.1039/d1sc01806j |
Appears in Collections: | Aurora harvest 8 Chemistry publications |
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hdl_131416.pdf | 2.44 MB | Adobe PDF | View/Open |
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